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国家自然科学基金(20621140004)

作品数:2 被引量:16H指数:2
相关作者:刘畅薛莉贺泓更多>>
相关机构:中国科学院生态环境研究中心更多>>
发文基金:国家自然科学基金国家重点基础研究发展计划更多>>
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Combination of biodiesel-ethanol-diesel fuel blend and SCR catalyst assembly to reduce emissions from a heavy-duty diesel engine被引量:8
2008年
In this study, the efforts to reduce NOx and particulate matter (PM) emissions from a diesel engine using both ethanol-selective catalytic reduction (SCR) of NOx over an Ag/Al2O3 catalyst and a biodiesel-ethanol-diesel fuel blend (BE-diesel) on an engine bench test are discussed. Compared with diesel fuel, use of BE-diesel increased PM emissions by 14% due to the increase in the soluble organic fraction (SOF) of PM, but it greatly reduced the Bosch smoke number by 60%-80% according to the results from 13-mode test of European Stationary Cycle (ESC) test. The SCR catalyst was effective in NOx reduction by ethanol, and the NOx conversion was approximately 73%. Total hydrocarbons (THC) and CO emissions increased significantly during the SCR of NOx process. Two diesel oxidation catalyst (DOC) assemblies were used after Ag/Al2O3 converter to remove CO and HC. Different oxidation catalyst showed opposite effect on PM emission. The PM composition analysis revealed that the net effect of oxidation catalyst on total PM was an integrative effect on SOF reduction and sulfate formation of PM. The engine bench test results indicated that the combination of BE-diesel and a SCR catalyst assembly could provide benefits for NOx and PM emissions control even without using diesel particle filters (DPFs).
SHI XiaoyanYU YunboHE HongSHUAI ShijinDONG HongyiLI Rulong
碱金属及碱土金属对钴铈复合氧化物催化剂催化N2O分解的影响
采用柠檬酸络合法制备了添加不同碱金属及碱土金属的钴铈复合氧化物(Ce与Co物质的量比为0.05)催化剂,考察了其催化N2O分解的活性。结果表明,碱金属及碱土金属对钴铈催化剂催化N2O分解的活性均有促进作用,助催化效果递变...
薛莉刘畅贺泓
关键词:碱金属碱土金属CO3O4CEO2
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碱土金属对钴铈复合氧化物催化剂催化N_2O分解的影响被引量:8
2009年
采用低温柠檬酸络合法制备了添加不同碱土金属的钴铈复合氧化物(Ce/Co摩尔比为0.05)催化剂,考察了其催化N2O分解的活性.结果表明,碱土金属对钴铈催化剂催化N2O分解的活性有明显促进作用,助催化效果递变顺序为Mg
刘畅薛莉贺泓
关键词:碱土金属四氧化三钴二氧化铈复合氧化物催化剂
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