To improve the slab quality, a kind of non-sinusoidal oscillation technique of mold driven by elliptic gears was developed. The waveform functions of non-sinusoidal oscillation were determined, and the calculation method and curves of technological parameters for non-sinusoidal oscillation were given. At the case of waveform deviation factor a equal to 0.31 and oscillation amplitude h equal to ±2.7 mm, the relationship between oscillation frequency and casting speed is determined, and the technological parameters for non-sinusoidal oscillation are calculated. The testing results of industrial application indicated that this technique could not only improve the Slab surface quality, but also reduce the steel breakout.